Getting good at CSS3 animations and transitions takes practise. The only way to become proficient is by spending hours of working through different examples. Here are a number of good tutorials that generate some great effects.
CSS3 Navigation effect
http://www.alessioatzeni.com/blog/css3-menu-navigation-effect/
Animated Buttons
http://tympanus.net/codrops/2011/11/07/animated-buttons-with-css3/
Animated Bubble Buttons
http://tutorialzine.com/2010/10/css3-animated-bubble-buttons/
3D Image Gallery
http://inspectelement.com/tutorials/create-a-css3-image-gallery-with-a-3d-lightbox-animation/
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